[Back to Contents Page]

 

Mini-Reviews in Medicinal Chemistry, Volume 2, No. 4, 2002

 

Contents

 

Executive Editor: J.C. Hervé

Membranes as Barriers for Drug Design

 

Biomembrane Permeability of Peptides: Strategies to Improve Their Mucosal Uptake Pp.295-305

Andreas Bernkop-Schnürch and Andreas E. Clausen

[Abstract]

 

Cell Membranes As Barriers for The Use of Antisense Therapeutic Agents Pp.307-318

Ilpo Jääskeläinen and Arto Urtti

[Abstract]

 

Liposomes for Intravenous Drug Targeting: Design and Applications Pp.319-329

Josbert M. Metselaar, Enrico Mastrobattista and Gert Storm

[Abstract]

 

Membranes as Targets for Drug Design

 

How Do Channel- and Pore-Forming Helical Peptides Interact with Lipid Membranes and How does this Account for their Antimicrobial  Activity? Pp.331-342

Hervé Duclohier

[Abstract]

 

The Biochemical and Physiological Characteristics of Surface Receptors of Gram Negative Bacteria Pp.343-351

Lucienne Letellier and Mónica Santamaria

[Abstract]

 

Cytosolic Calcium Oscillations in Signal Transduction Pathways Pp.353-360

Michel F. Rossier and Alessandro M. Capponi

[Abstract]

 

Heterotrimeric G Proteins Control Diverse Pathways of Transmembrane Signaling, a Base for Drug Discovery Pp.361-372

Yves Landry and Jean-Pierre Gies

[Abstract]

 

Structure, Function and Modulation of Chemokine Receptors: Members of the G-Protein-Coupled Receptor Superfamily Pp.373-383

Ziwei Huang

[Abstract]

 

Molecular and Physicochemical Aspects of Local Anesthetics Acting on  Nicotinic Acetylcholine Receptor-containing Membranes Pp.385-410

Hugo R. Arias and Michael P. Blanton

[Abstract]

 

Non-genomic Effects of Steroid Hormones on Membrane Channels Pp.411-417

Jean-Claude Hervé

[Abstract]

 

Nerve Membrane Ion Channels as the Target Site of Insecticides Pp.419-432

Toshio Narahashi

[Abstract]

 

Abstracts

 

[Back to top] Biomembrane Permeability of Peptides: Strategies to Improve Their Mucosal Uptake

Andreas Bernkop-Schnürch and Andreas E. Clausen

 

In order to gain a therapeutic response after mucosal administration peptide drugs have to permeate the absorption membrane based on the mucus layer (I) and the epithelial tissue (II ) in significant quantities.The peptide drug transport across the membrane can be improved by the use of mucolytic agents and the permeation enhancers. The generation of novel, more potent permeation enhancers, based on an improved knowledge of the absorption membrane in combination with the appropriate delivery systems will strongly  improve the bioavailability of mucosally applied peptide drugs.

 

[Back to top] Cell Membranes As Barriers for The Use of Antisense Therapeutic Agents

Ilpo Jääskeläinen and Arto Urtti

 

Antisense oligonucleotides are promising therapeutical agents for numerous diseases resulting from overexpression of genes, expression of mutant genes and viral infections. As most oligonucleotides are polyanions they can not readily pass cellular membranes in adequate amounts to show activity. Therefore, different types of carrier systems and modifications have been developed to enhance absorption and distribution at the level of tissues and cells. The current state of delivery systems will be reviewed with a major part devoted to the commonly used cationic lipids.

 

[Back to top] Liposomes for Intravenous Drug Targeting: Design and Applications

Josbert M. Metselaar, Enrico Mastrobattista and Gert Storm

 

Drug targeting with liposomes has been studied for over 25 years and has demonstrated its value in clinical practice. This mini review offers an overview of the design and application of liposomes for i.v. drug targeting. Two approaches are outlined: passive and active targeting. The former approach is based on liposomes with prolonged circulation and selective target localization properties, while in the latter approach specific targeting ligands are coupled to the liposome surface in order to achieve enhanced interaction with target cell membranes.

 

[Back to top] How Do Channel- and Pore-Forming Helical Peptides Interact with Lipid Membranes and How does this Account for their Antimicrobial Activity?

Hervé Duclohier

 

Animals and plants defend themselves against pathogenic micro-organisms by the rapid mobilization of polycationic helical amphipathic peptides. Interactions with membranes induce optimal orientation and mutual structural changes, allowing for example to form transbilayer ion channels or pores whose properties are compared in this review. Physicochemical studies of peptide-lipid interactions provide attractive approaches for drug design.

 

[Back to top] The Biochemical and Physiological Characteristics of Surface Receptors of Gram Negative Bacteria

Lucienne Letellier and Mónica Santamaria

 

This review focuses on the properties of ferric iron surface receptors of Gram negative bacteria. We discuss the different strategies to acquire iron, and the fundamental role of these receptors in pathogenicity. The structure of some of these receptors, iron transport and regulation mechanisms are presented here.

 

[Back to top] Cytosolic Calcium Oscillations in Signal Transduction Pathways

Michel F. Rossier and Alessandro M. Capponi

 

The oscillatory nature of the intracellular calcium signal has been recognized as soon as the methodological developments allowed us to record calcium fluctuations at the single cell level. While the principal mechanisms responsible for the generation of these oscillations have been partially resolved, more attention has been recently focused on signal decoding and more particularly on the role of cell structure organization in transducing this signal to the molecular targets of the calcium messenger.

 

[Back to top] Heterotrimeric G Proteins Control Diverse Pathways of Transmembrane Signaling, a Base for Drug Discovery

Yves Landry and Jean-Pierre Gies

 

Heptahelical receptors are coupled to heterotrimeric GTP-binding proteins (G proteins) which transduce most signals through their a and bg subunits to effectors including adenylylcyclases, ion channels, phospholipases Cb, and phosphoinositide 3-kinases. The diversity of G proteins, their effectors and regulators (RGS proteins), supports the interest of these protein families as potential drug targets.

 

[Back to top] Structure, Function and Modulation of Chemokine Receptors: Members of the G-Protein-Coupled Receptor Superfamily

Ziwei Huang

 

Chemokine receptors are membrane proteins that play an important role in inflammation and the cellular entry of human immunodeficiency virus type I (HIV-1). Understanding the structure-function relationship of chemokine receptor-ligand interactions and developing novel strategies to control these interactions have important implications for therapeutic intervention of human diseases such as HIV-1 infection. This article reviews the work carried out in our laboratory in molecular modeling and site-directed mutagenesis of chemokine receptor-ligand interactions and chemical synthesis of chemokine-derived peptide agonists and antagonists. These studies demonstrate a paradigm for exploring and controlling membrane protein-protein interactions.

 

[Back to top] Molecular and Physicochemical Aspects of Local Anesthetics Acting on  Nicotinic Acetylcholine Receptor-containing Membranes

Hugo R. Arias and Michael P. Blanton

 

Local anesthetics inhibit the ion channel activity of nicotinic acetylcholine receptors in a noncompetitive fashion. This inhibitory action is ascribed to two possible inhibitory mechanisms: an openchannel- blocking mechanism and/or an allosteric process where the drug binds either to the closed channel or to other nonluminal sites, respectively.

 

[Back to top] Non-genomic Effects of Steroid Hormones on Membrane Channels

Jean-Claude Hervé

 

Steroid hormones may possess two distinct actions, a delayed genomic influence and the rapid nongenomic effects, which may act in concert. Nongenomic effect may be mediated by putative membrane receptors or due to allosteric interactions of steroids with membrane proteins (e.g. ionic channels), inducing rapid changes in protein/receptor/channel activation or inhibition.

 

[Back to top] Nerve Membrane Ion Channels as the Target Site of Insecticides

Toshio Narahashi

 

Most insecticides are potent neurotoxicants that act on various neuroreceptors and ion channels.However, the major target receptors are limited to sodium channels, GABA receptors, and nicotinic acetylcholine receptors. DDT and pyrethroids act similarly on sodium channels to keep them open leading to hyperexcitation. Indoxacarb inhibits sodium channels and certain subtypes of nicotinic receptors. Dieldrin,lindane and fipronil block GABA receptors. Imidacloprid modulates nicotinic receptors in a complex manner. Spinosad’s major target site appears to be nicotinic receptors.